Been forever since I've poked car audio, but yea, get a test album that plays a single frequency per track and work your way through it killing the rattles as you go. Of course, assuming it's rattles caused by car movement instead of the stereo that you're testing with, that might not be as effective unless you have a stereo that can really move shit around. Could always drop a big external speaker in temporarily if you really wanted to deal with it, although might be worth noting that some rattles might be caused by higher frequencies than a normal sub's crossover.